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Semiconducting Double-Layer Lead Monoxide Tin Oxide Nanostructures for Photodetectors

dc.contributor.authorAkay, Defne
dc.contributor.authorSeven, Elanur
dc.contributor.authorGokmen, Ugur
dc.contributor.authorBilge Ocak, Sema
dc.date.accessioned2026-10-09T21:48:56Z
dc.date.issued2023
dc.departmentYüksek İhtisas Üniversitesi
dc.description.abstractThis study examines the high-frequency-dependent characteristics of the PbO/SnO2 double-layer semiconductor (DLS) structures. Recently, researchers have been particularly interested in such structures in terms of their use in electrical and photovoltaic applications. A PbO/SnO2 double layer was successfully coated on a p-type Si substrate (100) wafer with a resistance of 10 ohm cm and a thickness of 280 mu m. The Al Schottky (round dot) connections, which have a thickness of 124 nm and a diameter of 1.3 mm, were produced by thermal evaporation. The present study proposes to measure the conductance-voltage (G-V) and capacitance-voltage (C-V) values of the studied Al/PbO/SnO2/p-Si Schottky diode for the frequencies of 500 kHz, 800 kHz, and 1 MHz at a temperature of 300 K, which has been suggested for the first time in literature. Due to the presence of surface states (N-ss), PbO/SnO2 double-layer, and series resistance R-s, the C-V and G-V plots show inversion, depletion, and accumulation zones depending on the strong frequency for each frequency tested. Based on the tested frequencies, the reverse-biased C-2-V curves are used to compute the fundamental electrical characteristics of the Al/PbO/SnO2/p-Si structures, including the depletion layer (W-D), Fermi energy level (E-F), diffusion potential (V-D), and thickness barrier height (circle divide(B)). We also investigated the capacitance features and the energy density distribution of surface states (N-ss) in the PbO/SnO2 double-layer structure by utilizing the measured values of G-V and C-V. The values of circle divide(B), V-D, and N-ss were observed to be 0.54 0.34, and 3.19 10 12 eV(-1) cm(-2) at 500 kHz, while they were 0.88 0.68, and 1.96 eV(-1) cm(-2) at 800 kHz and 0.95, 0.75, and 1.47 eV(-1) cm(-2) at 1 MHz, respectively. It was discovered that the capacitance characteristics of the PbO/SnO2 double-layer structure were substantially dependent on the applied high frequencies. Furthermore, the C-V and G-V measurements revealed that the series resistance and the interface state density of the studied Al/PbO/SnO2/p-Si Schottky diode were critical parameters that significantly affect the electrical parameters offered by the PbO/SnO2 double-layer nanostructure. The results of the study reveal that the manufactured device exhibits outstanding electric characteristics and support the possibility of using DL thin films in electronic devices.
dc.description.sponsorshipScientific Research Projects Office of Gazi University [FGA-2023-8522]
dc.description.sponsorshipThis study (Project No. FGA-2023-8522) has received financial aid from the Scientific Research Projects Office of Gazi University. The authors would like to state their sincere gratitude for their support.
dc.identifier.doi10.1021/acsanm.3c02610
dc.identifier.endpage17490
dc.identifier.issn2574-0970
dc.identifier.issue19
dc.identifier.orcid0000-0002-0590-7555
dc.identifier.scopus2-s2.0-85175006321
dc.identifier.scopusqualityQ1
dc.identifier.startpage17482
dc.identifier.urihttps://doi.org/10.1021/acsanm.3c02610
dc.identifier.urihttps://hdl.handle.net/20.500.12794/3597
dc.identifier.volume6
dc.identifier.wosWOS:001068825100001
dc.identifier.wosqualityQ2
dc.indekslendigikaynakWeb of Science
dc.indekslendigikaynakScopus
dc.indekslendigikaynak.digerScience Citation Index Expanded (SCI-EXPANDED)
dc.language.isoen
dc.publisherAmer Chemical Soc
dc.relation.ispartofAcs Applied Nano Materials
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı
dc.relation.sdgGoal-07: Affordable and Clean Energy
dc.rightsinfo:eu-repo/semantics/openAccess
dc.snmzKA_WoS_20260922
dc.subjectDouble-Layer Film
dc.subjectTin Oxide
dc.subjectLead Oxide
dc.subjectSchottky Diode
dc.subjectInterface States
dc.titleSemiconducting Double-Layer Lead Monoxide Tin Oxide Nanostructures for Photodetectors
dc.typeArticle

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